Advanced Search
WANG Zhe, WANG Zifa, LI Jie, ZHENG Haitao, YAN Pingzhong, LI Jianjun. Development of a Meteorology-Chemistry Two-Way Coupled Numerical Model (WRF-NAQPMS) and Its Application in a Severe Autumn Haze Simulation over the Beijing-Tianjin-Hebei Area, China[J]. Climatic and Environmental Research, 2014, 19(2): 153-163. doi: 10.3878/j.issn.1006-9585.2014.13231
Citation: WANG Zhe, WANG Zifa, LI Jie, ZHENG Haitao, YAN Pingzhong, LI Jianjun. Development of a Meteorology-Chemistry Two-Way Coupled Numerical Model (WRF-NAQPMS) and Its Application in a Severe Autumn Haze Simulation over the Beijing-Tianjin-Hebei Area, China[J]. Climatic and Environmental Research, 2014, 19(2): 153-163. doi: 10.3878/j.issn.1006-9585.2014.13231

Development of a Meteorology-Chemistry Two-Way Coupled Numerical Model (WRF-NAQPMS) and Its Application in a Severe Autumn Haze Simulation over the Beijing-Tianjin-Hebei Area, China

doi: 10.3878/j.issn.1006-9585.2014.13231
  • Received Date: 2013-12-23
  • Rev Recd Date: 2014-02-10
  • An aerosol-optical module based on Mie scattering theory has been implemented in the Nested Air Quality Prediction Modeling System (NAQPMS), and a new coupler has been developed to deal with the interaction between the mesoscale meteorology model WRF (Weather Research and Forecasting Model) and NAQPMS. The one-way off-line and two-way coupled WRF-NAQPMS models are compared to simulate the severe haze in the Beijing-Tianjin-Hebei area from 27 September to 1 October 2013. The results show that the simulated meteorological elements and PM2.5 concentrations from the two-way coupled model with the aerosol direct radiation effect are more consistent with observations. During the haze period, the boundary layer meteorological elements change significantly because of the aerosol direct radiation effect over the Beijing-Tianjin-Hebei area: Incoming solar radiation is reduced by 25%, the 2-m temperature decreases by 1 ℃, the turbulent kinetic energy is reduced by 25%, the 10-m wind speed decreases by up to 0.2 m/s, and the planetary boundary layer (PBL) height is reduced by 25%. These changes make the atmospheric boundary layer more stable and further exacerbate air pollution over the areas where it is already severe, for example, the PM2.5 concentration increases by up to 30% over Shijiazhuang City. The analysis indicates that there is a positive feedback mechanism between haze and boundary layer meteorology, and the two-way coupled model incorporating this feedback is helpful for accurate simulation and forecasting of haze pollution processes.
  • loading
  • [1]
    An X, Zhu T, Wang Z, et al. 2007. A modeling analysis of a heavy air pollution episode occurred in Beijing [J]. Atmospheric Chemistry and Physics, 7 (12): 3103-3114.
    [2]
    Barnard J C, Fast J D, Paredes-Miranda G, et al. 2010. Evaluation of the WRF-Chem “Aerosol Chemical to Aerosol Optical Properties” module using data from the MILAGRO campaign [J]. Atmospheric Chemistry and Physics, 10 (15): 7325-7340.
    [3]
    Li J, Wang Z, Wang X, et al. 2011. Impacts of aerosols on summertime tropospheric photolysis frequencies and photochemistry over central eastern China [J]. Atmos. Environ., 45 (10): 1817-1829.
    [4]
    Li J, Wang Z, Zhuang G, et al. 2012. Mixing of Asian mineral dust with anthropogenic pollutants over East Asia: A model case study of a super-duststorm in March 2010 [J]. Atmospheric Chemistry and Physics, 12 (16): 7591-7607.
    [5]
    Li J, Wang Z F, Huang H L, et al. 2013. Assessing the effects of trans- boundary aerosol transport between various city clusters on regional haze episodes in spring over East China [J]. Tellus B, 65, doi: 10.3402/tellusb. v65i0.20052.
    [6]
    Nenes A, Pandis S N, Pilinis C. 1998. ISORROPIA: A new thermodynamic equilibrium model for multiphase multicomponent inorganic aerosols [J]. Aquatic Geochemistry, 4 (1): 123-152.
    [7]
    Petters M D, Kreidenweis S M. 2007. A single parameter representation of hygroscopic growth and cloud condensation nucleus activity [J]. Atmospheric Chemistry and Physics, 7 (8): 1961-1971.
    [8]
    Quan J N, Gao Y, Zhang Q, et al. 2013. Evolution of planetary boundary layer under different weather conditions, and its impact on aerosol concentrations [J]. Particuology, 11 (1): 34-40.
    [9]
    Seinfeld J H, Pandis S N. 1998. Atmospheric Chemistry and Physics [M]. New York: John Wiley and Sons, Inc.
    [10]
    Skamarock W C, Klemp J B, Dudhia J, et al. 2008. A description of the Advanced Research WRF version 3 [R]. National Center for Atmospheric Research Tech. Note, NCAR/TN-475+STR, 113pp.
    [11]
    Stern R, Builtjes P, Schaap M, et al. 2008. A model inter-comparison study focussing on episodes with elevated PM10 concentrations [J]. Atmos. Environ., 42 (19): 4567-4588.
    [12]
    Tang X, Zhu J, Wang Z F, et al. 2011. Improvement of ozone forecast over Beijing based on ensemble Kalman filter with simultaneous adjustment of initial conditions and emissions [J]. Atmospheric Chemistry and Physics, 11 (24): 12901-12916.
    [13]
    Wang Z F, Maeda T, Hayashi M, et al. 2001. A nested air quality prediction modeling system for urban and regional scales: Application for high-ozone episode in Taiwan [J]. Water, Air, and Soil Pollution, 130 (1-4): 391-396.
    [14]
    Wang Z F, Akimoto H, Uno I. 2002. Neutralization of soil aerosol and its impact on the distribution of acid rain over East Asia: Observations and model results [J]. J. Geophys. Res., 107 (D19): ACH 6-1-ACH 6-12.
    [15]
    Wang Z F, Li J, Wang X Q, et al. 2006. Modeling of regional high ozone episode observed at two mountain sites (Mt. Tai and Huang) in East China [J]. Journal of Atmospheric Chemistry, 55 (3): 253-272.
    [16]
    王自发, 谢付莹, 王喜全, 等. 2006. 嵌套网格空气质量预报模式系统的发展与应用 [J]. 大气科学, 30 (5): 778-790. Wang Zifa, Xie Fuying, Wang Xiquan, et al. 2006. Development and application of nested air quality prediction modeling system [J]. Chinese Journal of Atmospheric Sciences (in Chinese), 30 (5): 778-790, doi: 10.3878/j.issn. 1006-9895. 2006.05.07.
    [17]
    Wong D C, Pleim J, Mathur R, et al. 2012. WRF-CMAQ two-way coupled system with aerosol feedback: Software development and preliminary results [J]. Geoscientific Model Development, 5 (2): 299-312, doi: 10.5194/gmd-5-299-2012.
    [18]
    Wu Q Z, Wang Z F, Gbaguidi A, et al. 2011. A numerical study of contributions to air pollution in Beijing during CAREBeijing-2006 [J]. Atmospheric Chemistry and Physics, 11 (12): 5997-6011.
    [19]
    Wu Z J, Hu M, Lin P, et al. 2008. Particle number size distribution in the urban atmosphere of Beijing, China [J]. Atmos. Environ., 42 (34): 7967-7980.
    [20]
    Zaveri R A, Peters L K. 1999. A new lumped structure photochemical mechanism for large-scale applications [J]. J. Geophys. Res., 104 (D23): 30387-30415.
    [21]
    Zhang Y, Wen X Y, Jang C J. 2010. Simulating chemistry-aerosol-cloud-radiation-climate feedbacks over the continental U.S. using the online-coupled Weather Research Forecasting Model with chemistry (WRF/Chem) [J]. Atmos. Environ., 44 (29): 3568- 3582.
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索

    Article Metrics

    Article views (7563) PDF downloads(6761) Cited by()
    Proportional views
    Related

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return