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Volume 6 Issue 1

Jan.  1989

Article Contents

Numerical Simulation on the Rainout-Removal of Sulfur Dioxide and Acidification of Precipitation from Stratiform Clouds


doi: 10.1007/BF02656919

  • The rainout-removal of SO2 and the acidification of precipitation from stratiform clouds are simulated using a one-dimensional, time-dependent model, parameterized microphysically in which dissolution and dissociation of gaseous SO2 and H2O2, and oxidation reaction in aqueous phase are taken into account. The effects of dynamic fac-tors, including updraft flow and turbulent transport, and the concentration of gaseous SO2 and H2O2 being transported into the clouds on pH value of the precipitation, the conversion rate S(IV)-S (VI) and the wet deposition rate of SO2 are discussed.
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    [2] Jiangbo JIN, Duoying JI, Xiao DONG, Kece FEI, Run GUO, Juanxiong HE, Yi YU, Zhaoyang CHAI, He ZHANG, Dongling ZHANG, Kangjun CHEN, Qingcun ZENG, 2024: CAS-ESM2.0 Dataset for the Carbon Dioxide Removal Model Intercomparison Project (CDRMIP), ADVANCES IN ATMOSPHERIC SCIENCES, 41, 989-1000.  doi: 10.1007/s00376-023-3089-3
    [3] LIU Xiaoli, NIU Shengjie, 2010: Numerical Simulation of Macro- and Micro-structures of Intense Convective Clouds with a Spectral Bin Microphysics Model, ADVANCES IN ATMOSPHERIC SCIENCES, 27, 1078-1088.  doi: 10.1007/s00376-010-8088-5
    [4] Yuqiang SONG, Hongnian LIU, Xueyuan WANG, Ning ZHANG, Jianning SUN, 2016: Numerical Simulation of the Impact of Urban Non-uniformity on Precipitation, ADVANCES IN ATMOSPHERIC SCIENCES, 33, 783-793.  doi: 10.1007/s00376-016-5042-1
    [5] Lei Xiao’en, Jia Xinyuan, Yuan Suzhen, Luo Qiren, Chen Silong, Xu Yu, 1987: A NUMERICAL SIMULATION OF THE DISTRIBUTION OF ACID PRECIPITATION IN CHONGQING AREA OF CHINA, ADVANCES IN ATMOSPHERIC SCIENCES, 4, 313-322.  doi: 10.1007/BF02663601
    [6] Tuanjie HOU, Hengchi LEI, Youjiang HE, Jiefan YANG, Zhen ZHAO, Zhaoxia HU, 2021: Aircraft Measurements of the Microphysical Properties of Stratiform Clouds with Embedded Convection, ADVANCES IN ATMOSPHERIC SCIENCES, 38, 966-982.  doi: 10.1007/s00376-021-0287-8
    [7] Yuanyuan ZUO, Zhiqun HU, Shujie YUAN, Jiafeng ZHENG, Xiaoyan YIN, Boyong LI, 2022: Identification of Convective and Stratiform Clouds Based on the Improved DBSCAN Clustering Algorithm, ADVANCES IN ATMOSPHERIC SCIENCES, 39, 2203-2212.  doi: 10.1007/s00376-021-1223-7
    [8] LI Weiping, XUE Yongkang, 2005: Numerical Simulation of the Impact of Vegetation Index on the Interannual Variation of Summer Precipitation in the Yellow River Basin, ADVANCES IN ATMOSPHERIC SCIENCES, 22, 865-876.  doi: 10.1007/BF02918686
    [9] Suping NIE, Tongwen WU, Yong LUO, Xueliang DENG, Xueli SHI, Zaizhi WANG, Xiangwen LIU, Jianbin HUANG, 2016: A Strategy for Merging Objective Estimates of Global Daily Precipitation from Gauge Observations, Satellite Estimates, and Numerical Predictions, ADVANCES IN ATMOSPHERIC SCIENCES, 33, 889-904.  doi: 10.1007/s00376-016-5223-y
    [10] Yafei YAN, Yimin LIU, 2019: Vertical Structures of Convective and Stratiform Clouds in Boreal Summer over the Tibetan Plateau and Its Neighboring Regions, ADVANCES IN ATMOSPHERIC SCIENCES, 36, 1089-1102.  doi: 10.1007/s00376-019-8229-4
    [11] Dejun LI, Chuanfeng ZHAO, Peiren LI, Cao Liu, Dianli GONG, Siyao LIU, Zhengteng YUAN, Yingying CHEN, 2022: Macro- and Micro-physical Characteristics of Different Parts of Mixed Convective-stratiform Clouds and Differences in Their Responses to Seeding, ADVANCES IN ATMOSPHERIC SCIENCES, 39, 2040-2055.  doi: 10.1007/s00376-022-2003-8
    [12] Tuanjie HOU, Baojun CHEN, Hengchi LEI, Lei WEI, Youjiang HE, Qiujuan FENG, 2023: Evaluation of the Predicted Particle Properties (P3) Microphysics Scheme in Simulations of Stratiform Clouds with Embedded Convection, ADVANCES IN ATMOSPHERIC SCIENCES, 40, 1859-1876.  doi: 10.1007/s00376-023-2178-7
    [13] Dongxu YANG, Yi LIU, Zhaonan CAI, Xi CHEN, Lu YAO, Daren LU, 2018: First Global Carbon Dioxide Maps Produced from TanSat Measurements, ADVANCES IN ATMOSPHERIC SCIENCES, 35, 621-623.  doi: 10.1007/s00376-018-7312-6
    [14] Dongxu YANG, Yi LIU, Liang FENG, Jing WANG, Lu YAO, Zhaonan CAI, Sihong ZHU, Naimeng LU, Daren LYU, 2021: The First Global Carbon Dioxide Flux Map Derived from TanSat Measurements, ADVANCES IN ATMOSPHERIC SCIENCES, 38, 1433-1443.  doi: 10.1007/s00376-021-1179-7
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    [17] Yongjie HUANG, Yaping WANG, Xiaopeng CUI, 2019: Differences between Convective and Stratiform Precipitation Budgets in a Torrential Rainfall Event, ADVANCES IN ATMOSPHERIC SCIENCES, 36, 495-509.  doi: 10.1007/s00376-019-8159-1
    [18] Bangjun Cao, Xianyu Yang, JUN WEN, Qin Hu, Ziyuan Zhu, 2023: Large eddy simulation of vertical structure and size distribution of deep layer clouds, ADVANCES IN ATMOSPHERIC SCIENCES.  doi: 10.1007/s00376-023-3134-2
    [19] Xiquan DONG, 2018: Preface to the Special Issue: Aerosols, Clouds, Radiation, Precipitation, and Their Interactions, ADVANCES IN ATMOSPHERIC SCIENCES, 35, 133-134.
    [20] XIE Baohua, ZHOU Zaixing, ZHENG Xunhua, ZHANG Wen, ZHU Jianguo, 2010: Modeling Methane Emissions from Paddy Rice Fields under Elevated Atmospheric Carbon Dioxide Conditions, ADVANCES IN ATMOSPHERIC SCIENCES, 27, 100-114.  doi: 10.1007/s00376-009-8178-4

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Manuscript History

Manuscript received: 10 January 1989
Manuscript revised: 10 January 1989
通讯作者: 陈斌, bchen63@163.com
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Numerical Simulation on the Rainout-Removal of Sulfur Dioxide and Acidification of Precipitation from Stratiform Clouds

  • 1. Department of Geophysics, Peking University, Beijing

Abstract: The rainout-removal of SO2 and the acidification of precipitation from stratiform clouds are simulated using a one-dimensional, time-dependent model, parameterized microphysically in which dissolution and dissociation of gaseous SO2 and H2O2, and oxidation reaction in aqueous phase are taken into account. The effects of dynamic fac-tors, including updraft flow and turbulent transport, and the concentration of gaseous SO2 and H2O2 being transported into the clouds on pH value of the precipitation, the conversion rate S(IV)-S (VI) and the wet deposition rate of SO2 are discussed.

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