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Volume 3 Issue 4

Oct.  1986

Article Contents

METEOROLOGICAL AND CHEMICAL CONTROLS ON THE VERTICAL DISTRIBUTION OF BEIJING SUMMER COARSE AND FINE AEROSOLS


doi: 10.1007/BF02657933

  • Vertical profiles of fine and coarse aerosol particles were determined by cascade impactors at the me-teorological tower in Beijing for three days and one night, July 18-23, 1980. Coarse mode aerosols showed a maximum concentration at 47 m when there was an inversion at about 140 m height, and a rather uniform distribution when there was no inversion. This may indicate a two-component origin of coarse particles at the tower site, one being surface dust and the other being tall stack emissions. Fine mode aerosols showed more complex vertical profiles. Median particle size distributions of most metals were bimodal, indicating distinct coarse particle dispersion and fine accumulation mode processes. A chemical thermodynamic cal-culation indicates that fine mode Si can result from the reduction of silica to volatile SiO during coal combustion with limited air supply, a process which should release substantial amounts of carbon monoxide to the atmosphere.
  • [1] Zhang Renjian, Wang Mingxing, Fu Jianzhong, 2001: Preliminary Research on the Size Distribution of???Aerosols in Beijing, ADVANCES IN ATMOSPHERIC SCIENCES, 18, 225-230.  doi: 10.1007/s00376-001-0015-3
    [2] ZHANG Renjian, XU Yongfu, HAN Zhiwei, 2004: A Comparison Analysis of Chemical Composition of Aerosols in the Dust and Non-Dust Periods in Beijing, ADVANCES IN ATMOSPHERIC SCIENCES, 21, 300-305.  doi: 10.1007/BF02915718
    [3] WANG Yuesi, HU Bo, LIU Guangren, 2005: A Primary Study of the Variations of Vertical Radiation with the Beijing 325-m Meteorological Tower, ADVANCES IN ATMOSPHERIC SCIENCES, 22, 172-180.  doi: 10.1007/BF02918507
    [4] Ping LI, Siyao YUE, Xiaoyang YANG, Di LIU, Qiang ZHANG, Wei HU, Shengjie HOU, Wanyu ZHAO, Hong REN, Gang LI, Yuanguan GAO, Junjun DENG, Qiaorong XIE, Yele SUN, Zifa WANG, Pingqing FU, 2023: Fluorescence Properties and Chemical Composition of Fine Particles in the Background Atmosphere of North China, ADVANCES IN ATMOSPHERIC SCIENCES, 40, 1159-1174.  doi: 10.1007/s00376-022-2208-x
    [5] LI Xuxiang, CAO Junji, Judith CHOW, HAN Yongming, Shuncheng LEE, John WATSON, 2008: Chemical Characteristics of Carbonaceous Aerosols During Dust Storms over Xi'an in China, ADVANCES IN ATMOSPHERIC SCIENCES, 25, 847-855.  doi: 10.1007/s00376-008-0847-1
    [6] Chuanfeng ZHAO, Yanan LI, Fang ZHANG, Yele SUN, Pucai WANG, 2018: Growth Rates of Fine Aerosol Particles at a Site near Beijing in June 2013, ADVANCES IN ATMOSPHERIC SCIENCES, 35, 209-217.  doi: 10.1007/s00376-017-7069-3
    [7] Jun WANG, Jinming FENG, Qizhong WU, Zhongwei YAN, 2016: Impact of Anthropogenic Aerosols on Summer Precipitation in the Beijing-Tianjin-Hebei Urban Agglomeration in China: Regional Climate Modeling Using WRF-Chem, ADVANCES IN ATMOSPHERIC SCIENCES, 33, 753-766.  doi: 10.1007/s00376-015-5103-x
    [8] Su Weihan, Zhang Qiupeng, Song Wenzhi, R. L. Dod, R. D. Giauque, T. Novakov, 1987: PRIMARY STUDY OF SULFATE AND CARBONACEOUS AEROSOLS IN BEIJING, ADVANCES IN ATMOSPHERIC SCIENCES, 4, 225-232.  doi: 10.1007/BF02677069
    [9] Chibuike Chiedozie IBEBUCHI, Cameron C. LEE, 2024: Circulation Pattern Controls of Summer Temperature Anomalies in Southern Africa, ADVANCES IN ATMOSPHERIC SCIENCES, 41, 341-354.  doi: 10.1007/s00376-023-2392-3
    [10] SUN Yang, WANG Yuesi, ZHANG Changchun, 2010: Vertical Observations and Analysis of PM2.5, O3, and NOx at Beijing and Tianjin from Towers during Summer and Autumn 2006, ADVANCES IN ATMOSPHERIC SCIENCES, 27, 123-136.  doi: 10.1007/s00376-009-8154-z
    [11] YANG Fumo, Jeffrey BROOK, HE Kebin, DUAN Fengkui, MA Yongliang, 2010: Temporal Variability in Fine Carbonaceous Aerosol over Two Years in Two Megacities: Beijing and Toronto, ADVANCES IN ATMOSPHERIC SCIENCES, 27, 705-714.  doi: 10.1007/s00376-009-9103-6
    [12] Zou Han, Zhou Libo, Jian Yongxiao, Liu Yu, 2002: An Observational Study on the Vertical Distribution and Synoptic Variation of Ozone in the Arctic, ADVANCES IN ATMOSPHERIC SCIENCES, 19, 855-862.  doi: 10.1007/s00376-002-0050-8
    [13] Bangjun Cao, Xianyu Yang, JUN WEN, Qin Hu, Ziyuan Zhu, 2023: Large eddy simulation of vertical structure and size distribution of deep layer clouds, ADVANCES IN ATMOSPHERIC SCIENCES.  doi: 10.1007/s00376-023-3134-2
    [14] ZHANG Junke, WANG Yuesi, HUANG Xiaojuan, LIU Zirui, JI Dongsheng, SUN Yang, 2015: Characterization of Organic Aerosols in Beijing Using an Aerodyne High-Resolution Aerosol Mass Spectrometer, ADVANCES IN ATMOSPHERIC SCIENCES, 32, 877-888.  doi: 10.1007/s00376-014-4153-9
    [15] Guo DENG, Xueshun SHEN, Jun DU, Jiandong GONG, Hua TONG, Liantang DENG, Zhifang XU, Jing CHEN, Jian SUN, Yong WANG, Jiangkai HU, Jianjie WANG, Mingxuan CHEN, Huiling YUAN, Yutao ZHANG, Hongqi LI, Yuanzhe WANG, Li GAO, Li SHENG, Da LI, Li LI, Hao WANG, Ying ZHAO, Yinglin LI, Zhili LIU, Wenhua GUO, 2024: Scientific Advances and Weather Services of the China Meteorological Administration’s National Forecasting Systems during the Beijing 2022 Winter Olympics, ADVANCES IN ATMOSPHERIC SCIENCES, 41, 767-776.  doi: 10.1007/s00376-023-3206-3
    [16] LIU Yu, LI Weiliang, ZHOU Xiuji, HE Jinhai, 2003: Mechanism of Formation of the Ozone Valley over the Tibetan Plateau in Summer Transport and Chemical Process of Ozone, ADVANCES IN ATMOSPHERIC SCIENCES, 20, 103-109.  doi: 10.1007/BF03342054
    [17] Ravidho RAMADHAN, MARZUKI, Mutya VONNISA, HARMADI, Hiroyuki HASHIGUCHI, Toyoshi SHIMOMAI, 2020: Diurnal Variation in the Vertical Profile of the Raindrop Size Distribution for Stratiform Rain as Inferred from Micro Rain Radar Observations in Sumatra, ADVANCES IN ATMOSPHERIC SCIENCES, 37, 832-846.  doi: 10.1007/s00376-020-9176-9
    [18] WU Xue*, WANG Xin, and LÜ Daren, 2014: Retrieval of Vertical Distribution of Tropospheric Refractivity through Ground-Based GPS Observation, ADVANCES IN ATMOSPHERIC SCIENCES, 31, 37-47.  doi: 10.1007/s00376-013-2215-z
    [19] Juan HUO, Yongheng BI, Daren Lü, Shu DUAN, 2019: Cloud Classification and Distribution of Cloud Types in Beijing Using Ka-Band Radar Data, ADVANCES IN ATMOSPHERIC SCIENCES, , 793-803.  doi: 10.1007/s00376-019-8272-1
    [20] LIU Dameng, GAO Shaopeng, AN Xianghua, 2008: Distribution and Source Apportionment of Polycyclic Aromatic Hydrocarbons from Atmospheric Particulate Matter PM2.5 in Beijing, ADVANCES IN ATMOSPHERIC SCIENCES, 25, 297-305.  doi: 10.1007/s00376-008-0297-9

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Manuscript History

Manuscript received: 10 October 1986
Manuscript revised: 10 October 1986
通讯作者: 陈斌, bchen63@163.com
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    沈阳化工大学材料科学与工程学院 沈阳 110142

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METEOROLOGICAL AND CHEMICAL CONTROLS ON THE VERTICAL DISTRIBUTION OF BEIJING SUMMER COARSE AND FINE AEROSOLS

  • 1. Institute of Atmospheric Physics, Academia Sinica, Beijing,Institute of Atmospheric Physics, Academia Sinica, Beijing,Institute of Atmospheric Physics, Academia Sinica, Beijing,Institute of Atmospheric Physics, Academia Sinica, Beijing,Institute of Atmospheric Physics, Academia Sinica, Beijing

Abstract: Vertical profiles of fine and coarse aerosol particles were determined by cascade impactors at the me-teorological tower in Beijing for three days and one night, July 18-23, 1980. Coarse mode aerosols showed a maximum concentration at 47 m when there was an inversion at about 140 m height, and a rather uniform distribution when there was no inversion. This may indicate a two-component origin of coarse particles at the tower site, one being surface dust and the other being tall stack emissions. Fine mode aerosols showed more complex vertical profiles. Median particle size distributions of most metals were bimodal, indicating distinct coarse particle dispersion and fine accumulation mode processes. A chemical thermodynamic cal-culation indicates that fine mode Si can result from the reduction of silica to volatile SiO during coal combustion with limited air supply, a process which should release substantial amounts of carbon monoxide to the atmosphere.

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