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Volume 15 Issue 3

Jul.  1998

Article Contents
Article >  ADVANCES IN ATMOSPHERIC SCIENCES  > 1998 >  15(3): 380-392

Seasonal and Spatial Variation of Radiative Effects of Anthropogenic Sulfate Aerosol

  • 1.

    START Regional Center for TEA, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029,START Regional Center for TEA, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029,START Regional Center for TEA, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029,START Regional Center for TEA, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029


doi: 10.1007/s00376-998-0008-6

  • On the basis of the emission data of the industrial sulphur dioxide (SO2) and observed climate fields over East Asia, the distribution of anthropogenic sulfate aerosol (SO) with seasonal variation in the troposphere is simulated and analyzed by a regional sulfur transport model, and the direct radiative effects of SO under different weather conditions are also calculated using the discrete ordinate method. The results show that the concentration of SO has significant seasonal and spatial variations resulting from the effects of SO2 emission source and precipita-tion and wind fields. Both the concentration of SO2 and its radiative forcing have the largest values in October and the lowest in July. SO causes the decrease of the radiation flux absorbed by earth-atmosphere and the cooling of air temperature by scattering more solar radiation back into space. Besides, the radiative and climatic effects of SO are related to the types and height and optical thickness, etc., of the clouds.
  • [1] Lingyun LOUSchool, of Earth, Zhejiang University, Xiaofan LISchool, 2016: Radiative Effects on Torrential Rainfall during the Landfall of Typhoon Fitow (2013), ADVANCES IN ATMOSPHERIC SCIENCES, 33, 101-109.  doi: 10.1007/s00376-015-5139-y
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    [3] ZHANG Hua, WANG Zhili, GUO Pinwen, WANG Zaizhi, 2009: A Modeling Study of the Effects of Direct Radiative Forcing Due to Carbonaceous Aerosol on the Climate in East Asia, ADVANCES IN ATMOSPHERIC SCIENCES, 26, 57-66.  doi: 10.1007/s00376-009-0057-5
    [4] Hu Rongming, Serge Planton, Michel Déque, Pascal Marquet, Alain Braun, 2001: Why Is the Climate Forcing of Sulfate Aerosols So Uncertain?, ADVANCES IN ATMOSPHERIC SCIENCES, 18, 1103-1120.  doi: 10.1007/s00376-001-0026-0
    [5] Min ZHAO, Tie DAI, Hao WANG, Qing BAO, Yimin LIU, Hua ZHANG, Guangyu SHI, 2022: Simulating Aerosol Optical Depth and Direct Radiative Effects over the Tibetan Plateau with a High-Resolution CAS FGOALS-f3 Model, ADVANCES IN ATMOSPHERIC SCIENCES, 39, 2137-2155.  doi: 10.1007/s00376-022-1424-8
    [6] SUN Zhian, WANG Xiaoyun, ZENG Xianning, 2006: Radiative Forcing of SO2 and NOx: A Case Study in Beijing, ADVANCES IN ATMOSPHERIC SCIENCES, 23, 317-322.  doi: 10.1007/s00376-006-0317-6
    [7] Huang Runheng, Kuo-Nan Liou, 1985: EFFECTS OF HORIZONTAL ORIENTATION ON THE RADIATIVE PROPERTIES OF ICE CLOUDS, ADVANCES IN ATMOSPHERIC SCIENCES, 2, 20-27.  doi: 10.1007/BF03179733
    [8] LIU Hongnian, ZHANG Li, WU Jian, 2010: A Modeling Study of the Climate Effects of Sulfate and Carbonaceous Aerosols over China, ADVANCES IN ATMOSPHERIC SCIENCES, 27, 1276-1288.  doi: 10.1007/s00376-010-9188-y
    [9] LI Jiandong, Zhian SUN, LIU Yimin, Jiangnan LI, Wei-Chyung WANG, WU Guoxiong, 2012: A Study on Sulfate Optical Properties and Direct Radiative Forcing Using LASG-IAP General Circulation Model, ADVANCES IN ATMOSPHERIC SCIENCES, 29, 1185-1199.  doi: 10.1007/s00376-012-1257-y
    [10] Yan XIA, Yongyun HU, Jiping LIU, Yi HUANG, Fei XIE, Jintai LIN, 2020: Stratospheric Ozone-induced Cloud Radiative Effects on Antarctic Sea Ice, ADVANCES IN ATMOSPHERIC SCIENCES, 37, 505-514.  doi: 10.1007/s00376-019-8251-6
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    [12] WANG Hong, SHI Guangyu, LI Shuyan, LI Wei, WANG Biao, HUANG Yanbin, 2006: The Impacts of Optical Properties on Radiative Forcing Due to Dust Aerosol, ADVANCES IN ATMOSPHERIC SCIENCES, 23, 431-441.  doi: 10.1007/s00376-006-0431-5
    [13] Li XU, Lin DU, Narcisse T. TSONA, Maofa GE, 2021: Anthropogenic Effects on Biogenic Secondary Organic Aerosol Formation, ADVANCES IN ATMOSPHERIC SCIENCES, 38, 1053-1084.  doi: 10.1007/s00376-020-0284-3
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    • Manuscript History

    Manuscript received: 10 July 1998
    Manuscript revised: 10 July 1998
    通讯作者: 陈斌, bchen63@163.com
    • 1. 

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    Seasonal and Spatial Variation of Radiative Effects of Anthropogenic Sulfate Aerosol

    • 1. START Regional Center for TEA, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029,START Regional Center for TEA, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029,START Regional Center for TEA, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029,START Regional Center for TEA, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029
    • Manuscript received: 1998-07-10
    • Manuscript revised: 1998-07-10

    Abstract: On the basis of the emission data of the industrial sulphur dioxide (SO2) and observed climate fields over East Asia, the distribution of anthropogenic sulfate aerosol (SO) with seasonal variation in the troposphere is simulated and analyzed by a regional sulfur transport model, and the direct radiative effects of SO under different weather conditions are also calculated using the discrete ordinate method. The results show that the concentration of SO has significant seasonal and spatial variations resulting from the effects of SO2 emission source and precipita-tion and wind fields. Both the concentration of SO2 and its radiative forcing have the largest values in October and the lowest in July. SO causes the decrease of the radiation flux absorbed by earth-atmosphere and the cooling of air temperature by scattering more solar radiation back into space. Besides, the radiative and climatic effects of SO are related to the types and height and optical thickness, etc., of the clouds.

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