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郑元媛, 韩志伟, 吴涧, 等. 2023. 中国地区生物质燃烧源排放的时空分布特征和排放清单比较[J]. 气候与环境研究, 28(5): 495−508. doi: 10.3878/j.issn.1006-9585.2022.22052
引用本文: 郑元媛, 韩志伟, 吴涧, 等. 2023. 中国地区生物质燃烧源排放的时空分布特征和排放清单比较[J]. 气候与环境研究, 28(5): 495−508. doi: 10.3878/j.issn.1006-9585.2022.22052
ZHENG Yuanyuan, HAN Zhiwei, WU Jian, et al. 2023. Spatial Distribution and Temporal Variation of Biomass Burning Emissions and Intercomparison of Biomass Burning Emission Inventories over China [J]. Climatic and Environmental Research (in Chinese), 28 (5): 495−508. doi: 10.3878/j.issn.1006-9585.2022.22052
Citation: ZHENG Yuanyuan, HAN Zhiwei, WU Jian, et al. 2023. Spatial Distribution and Temporal Variation of Biomass Burning Emissions and Intercomparison of Biomass Burning Emission Inventories over China [J]. Climatic and Environmental Research (in Chinese), 28 (5): 495−508. doi: 10.3878/j.issn.1006-9585.2022.22052

中国地区生物质燃烧源排放的时空分布特征和排放清单比较

Spatial Distribution and Temporal Variation of Biomass Burning Emissions and Intercomparison of Biomass Burning Emission Inventories over China

  • 摘要: 生物质燃烧向大气中排放大量痕量气体和颗粒物,源排放清单是深入研究生物质燃烧环境气候效应的重要基础数据。利用全球火排放数据库GFED(Global Fire Emissions Database)、NCAR全球火排放清单FINN(Fire INventory from NCAR)和中国露天生物质燃烧排放清单MEIC(Multi-resolution Emission Inventory for China),对2008~2017年中国地区生物质燃烧源排放的空间分布、季节和年际变化特征以及不同清单间的异同进行分析研究。3个清单都显示生物质燃烧释放的黑碳(BC)、有机碳(OC)、空气动力学粒径小于2.5 µm 的颗粒物(PM2.5)和一氧化碳(CO)在中国东北、长江和黄河下游之间地区和中国南方的排放量较高,与我国的主要农作物产地和森林地区分布一致。FINN清单排放量在华南地区与西南地区比其他两个清单高,而GFED清单排放量在长三角地区比其他两个清单排放量高。中国地区平均生物质燃烧排放量在春季出现峰值,而在不同的生物质燃烧地区峰值出现的季节不同,与各地农作物播种、收获时节和农耕习惯不同有关。2008~2017年,中国地区年平均生物质燃烧排放量的峰值主要出现在2014年,但各地区峰值出现的年份明显不同,东北、华中/东、华南和西南地区分别在2015年、2013年、2008年和2010年排放量达到最大。对于BC、OC和PM2.5,GFED和MEIC清单中的排放量比较接近,而FINN中的排放量是GFED和MEIC中的2~3倍;3个清单中CO的排放量比较接近。2014年生物质燃烧源排放与人为源排放的对比分析表明,所有物种中,生物质燃烧排放的OC和PM2.5相对于人为源排放量占比最大,3个清单中占比分别为9%~24%和5%~16%,说明生物质燃烧排放的OC和一次PM2.5是中国气溶胶的重要来源。

     

    Abstract: Biomass burning emits large amounts of trace gases and particulate matter into the atmosphere. Emission inventories are important datasets for studying the environmental and climatic effects of biomass burning. The spatial distribution, seasonal changes, and interannual variations in biomass burning emissions over China during 2008–2017 were investigated based on three biomass burning inventories, namely, the Global Fire Emissions Database (GFED), the Fire INventory from NCAR (FINN), and the emission inventory of open biomass burning in China (MEIC). The similarities and differences among the inventories were also compared and analyzed. The inventories consistently exhibited high amounts of black carbon (BC), organic carbon (OC), aerodynamic particulate matter with a size of <2.5 µm (PM2.5), and carbon monoxide (CO) from biomass burning over Northeast China, the regions between the lower reaches of the Yellow River and Yangtze River, and southern China, where agriculture and forest areas concentrated. The emission amounts in the FINN inventory were larger in southern and Southwest China than those in the other two inventories, whereas the emission amounts in the GFED inventory were higher in the Yangtze River Delta. Averaged over China, the peak of biomass burning emissions was in spring, whereas the peak emission amount occurred in different seasons for typical subregions of China, which could be related to different crop-sowing seasons and seeding habits. Between 2008 and 2017, the domain average annual biomass burning emissions peaked in 2014 in China. However, the period corresponding to maximum emissions was different for the subregions. Maximum emissions occurred in 2015, 2013, 2008, and 2010 in Northeast China, East China, South China, and Southwest China, respectively. For BC, OC, and PM2.5, the estimated domain average emissions over China were similar between GFED and MEIC, whereas the emissions in FINN were 2–3 times higher than those in the other two inventories. The CO emissions were similar in the three inventories. The annual and domain average OC and PM2.5 emissions from biomass burning in the three emission inventories accounted for 9%–24% and 5%–16%, respectively, of anthropogenic emissions over China in 2014, indicating that OC and primary PM2.5 from biomass burning are important sources of primary aerosols over China.

     

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