高级检索

青藏高原西部大气颗粒物污染特征及来源分析

Analysis of the Pollution Characteristics and Sources of Atmospheric Particulates in the Western Qinghai-Tibet Plateau

  • 摘要: 研究青藏高原大气颗粒物污染特征及其来源,对青藏高原生态环境保护、气候变化的影响及应对等领域具有重要的科学意义。本研究利用2019年7-8月第二次青藏科考在阿里的观测试验资料、阿里狮泉河国家气候站观测数据和GDAS1数据,采用源解析正定矩阵因子分解模型、后向轨迹距聚类、浓度权重轨迹分析等手段,分析了夏季青藏高原西部地区大气颗粒物污染特征、源区分布以及贡献。研究发现,夏季青藏高原西部阿里地区的总悬浮颗粒物(TSP)由沙尘、有机物、非粉尘水溶性无机离子、单质碳构成,贡献率分别为48.7%、12.7%、37.6%、0.9%。沙尘中的金属单质与风速呈正相关。高钾浓度和高有机碳与单质碳比(OC/EC)表明高原西部生物质燃烧的影响远大于化石燃料燃烧的影响。通过正定矩阵因子分解模型解析结果表明,夏季青藏高原西部主要有沙尘、二次生成、生物质燃烧、化石燃料燃烧、等四种污染来源,它们对总悬浮颗粒物(TSP)的贡献为38%、28%、27%、7%。自然排放的沙尘和生物质燃烧产生的人为有机气溶胶是青藏高原西部颗粒物的主要组成部分。采用后向轨迹距聚类和浓度权重轨迹分析发现,青藏高原西部地区的外来污染物主要来自南亚地区的短距离输送,尤其是印度西北部地区对青藏高原西部影响尤为明显。有机碳、单质碳、硫酸盐等人为排放气溶胶,塔尔沙漠的沙尘输送,以及印度生物质燃烧对青藏高原西部颗粒物浓度有显著影响,其中印度生物质燃烧影响最大。青藏高原西部的沙尘主要源于局地强风起沙,部分来自塔尔沙漠的输送,少量来自青藏高原北侧塔克拉玛干沙漠。

     

    Abstract: The study of atmospheric particulate matter pollution characteristics and their sources on the Tibetan Plateau is of great significance for the ecological environmental protection of the Tibetan Plateau and for the ability to cope with the adverse effects of climate change. In this paper, we analyze the characteristics of atmospheric particulate matter using observational data from the second Qinghai-Tibetan Science Expedition in Ali in July-August 2019, as well as observational data from the Ali Shiquanhe National Climate Station and GDAS1 data. The distribution of source areas and the degree of contribution of pollution to the western Tibetan Plateau in summer are analyzed using the source-resolved positive-definite matrix factor decomposition model, the backward trajectory-distance clustering, and the concentration-weighted trajectory analysis, among other techniques. The main conclusions are as follows: The TSP in the Ali region of the western Tibetan Plateau in summer is composed of sand and dust, organic matter, non-dust water-soluble inorganic ions, and singlet carbon. The pollution can be attributed to four main sources, namely sand and dust, secondary generation, biomass burning and fossil fuel combustion. The impact of biomass burning in the western part of the plateau is significantly greater than that of fossil fuel burning. The naturally emitted sand and dust, along with the anthropogenic organic aerosols from biomass burning, constitute the primary components of particulate matter in the western Tibetan Plateau. Notably, biomass burning in India has a considerable influence on the particulate matter concentrations in the western Tibetan Plateau.

     

/

返回文章
返回