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潘小乐, 王自发, 王喜全, 等. 秋季在北京城郊草地下垫面上的一次臭氧干沉降观测试验[J]. 大气科学, 2010, 34(1): 120-130. DOI: 10.3878/j.issn.1006-9895.2010.01.11
引用本文: 潘小乐, 王自发, 王喜全, 等. 秋季在北京城郊草地下垫面上的一次臭氧干沉降观测试验[J]. 大气科学, 2010, 34(1): 120-130. DOI: 10.3878/j.issn.1006-9895.2010.01.11
PAN Xiaole, WANG Zifa, WANG Xiquan, et al. An Observation Study of Ozone Dry Deposition over Grassland in the Suburban Area of Beijing[J]. Chinese Journal of Atmospheric Sciences, 2010, 34(1): 120-130. DOI: 10.3878/j.issn.1006-9895.2010.01.11
Citation: PAN Xiaole, WANG Zifa, WANG Xiquan, et al. An Observation Study of Ozone Dry Deposition over Grassland in the Suburban Area of Beijing[J]. Chinese Journal of Atmospheric Sciences, 2010, 34(1): 120-130. DOI: 10.3878/j.issn.1006-9895.2010.01.11

秋季在北京城郊草地下垫面上的一次臭氧干沉降观测试验

An Observation Study of Ozone Dry Deposition over Grassland in the Suburban Area of Beijing

  • 摘要: 2007年9月23日至10月13日, 在北京昌平区蟒山森林公园内, 利用浓度梯度观测法研究了秋季草地下垫面上臭氧的干沉降特征。研究结果表明: (1) 整个观测期间, 臭氧干沉降通量和干沉降速率平均值分别为-0.40 μg?m-2?s-1(负号表示方向指向地面) 和0.55 cm/s。 (2) 臭氧干沉降通量和干沉降速率受观测点山谷风的影响, 当白天谷风主导时, 臭氧的干沉降通量最大, 其平均值为-0.67 μg?m-2?s-1; 在山风、 谷风转换期间, 其平均值为-0.44 μg?m-2?s-1; 夜间山风主导时最小, 为-0.26 μg?m-2?s-1。臭氧干沉降速率也呈现同样的变化规律, 三种情形下的平均沉降速率分别为0.74 cm/s、 0.50 cm/s和0.47 cm/s。 (3) 利用阻力模型计算了臭氧的植被冠层阻力 (Rc), 结果表明: 由于白天植被的光合作用, 叶面气孔打开, 冠层阻力相对较小, Rc 的平均值为109.0 s/m; 夜间植被叶面气孔关闭, 阻力有明显升高, Rc的平均值为217.7 s/m; 在整个观测期间, Rc的平均值为184.0 s/m。

     

    Abstract: The field experiment of ozone dry deposition over grassland was performed by using the concentration gradient method in the suburban area of Beijing which is often situated downwind of urban plumes and then influenced by high ozone concentration episode. The vertical profiles of ozone concentration and meteorological parameters were measured in early autumn (23 September-13 October 2007) in a valley of Mangshan Forest Park. Strict data quality control procedures were performed to guarantee the credibility of following analysis. Results show that: (1) Both ozone flux and dry deposition velocity were characterized by strong diurnal variation, with daily mean values of -0.40 μg?m-2?s-1 (minus sign refers the direction towards the ground) and 0.55 cm/s respectively.(2) The ozone dry deposition flux is significantly influenced by the topographic wind, and the maximum ozone dry deposition flux occurs during the valley-wind prevailing period (0900-1500 LST) with a mean value of -0.67 μg?m-2?s-1, and it comes to averagely -0.44 μg?m-2?s-1 over the mountain-valley wind shift period (0800 LST in the morning and 1600 LST in the afternoon). When the observation site is predominated by mountain breeze, the downward ozone flux decreases to only -0.26 μg?m-2?s-1. The ozone dry deposition velocity displays the same feature with mean values of 0.74 cm/s, 0.50 cm/s, 0.47 cm/s respectively for these periods.(3) Canopy resistance calculated with the resistance model indicates the mean value of 184.0 s/m for the whole observation period. During the daytime, due to the gas-phase exchanges near leaf stomata and the strong photosynthesis effects, canopy resistance (109.0 s/m) is lower than that at night (217.7 s/m) when the plant physiological activities drop off.

     

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