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2003~2022年中国东北对流层大气甲烷浓度时空分布与地质排放影响研究

Study on Spatio–Temporal Distribution Mechanism of Methane Concentration and Geological Release Sources in the Atmospheric Troposphere across Northeast China during 2003–2022

  • 摘要: 中国东北存在中国最大的高纬度多年冻土分布带,随着全球气候变暖的加剧,多年冻土内储存的碳将逐渐解冻并以甲烷气体的形式释放,进而提高近地面对流层甲烷浓度,然而目前针对此区域近地面对流层甲烷浓度变化规律及排放源研究尚不清晰。本文利用Aqua卫星搭载的AIRS(Atmospheric InfraredSounder)遥感资料对中国东北及全国区域2003~2022年对流层整体甲烷浓度时空分布情况及变化趋势进行分析,并结合国家气象及现场监测数据,研究了中国东北多年冻土区地表甲烷排放源及排放机理。结果表明:中国东北地区多年冻土带在四季中均具有较高的甲烷排放能力,甲烷浓度呈显著的双峰季节变化特征,第一个峰值出现在夏季(6~8月),最大值出现在8月,第二个峰值出现在冬季(12~2月),最大值出现在12月;中国东北地区对流层甲烷浓度平均增长率最大值出现在春季(平均值为6.05 ppb/a,1 ppb=10-9),这是因为多年冻土退化后冻结层下封存的古老碳逐渐暴露并以甲烷的形式释放;除产甲烷菌作用,储存在多年冻土冻结层的地质甲烷(亚稳态甲烷水合物,稳态甲烷水合物及地下深处或煤层产生的产热甲烷)也逐渐被释放。最后,结合现场监测结果给出了多年冻土区地质甲烷热—气—固耦合作用模型,为中国东北多年冻土区碳循环研究提供数据和技术支持。

     

    Abstract: Northeast China has the largest high-latitude permafrost distribution regions in China. With the intensification of global warming, carbon stored in permafrost will gradually thaw and release in the form of methane gas, thereby increasing the concentration of methane in the troposphere. However, studies on changes in the methane concentration and release sources in the near-surface troposphere of this region are currently unclear. This paper analyzes the spatiotemporal distribution and change trend of the tropospheric methane concentration across China from 2003 to 2022 using the remote sensing data of Atmospheric InfraredSounder from Aqua satellite and studies the source and mechanism of surface methane release in the permafrost region of Northeast China in combination with the national meteorological and field monitoring data. Results show that the permafrost regions in Northeast China has a high methane release capacity in the four seasons, and the methane concentration presents a significant double-peak seasonal variation feature. The first peak appears in summer (June–August), where the maximum is observed in August. The second peak appears in winter (December–February), where the maximum is noticed in December. The maximum average growth rate of the tropospheric methane concentration in Northeast China appears in spring (the average value is 6.05 ppb/a, 1 ppb=10-9) because the carbon stored under the frozen layer is gradually exposed and released in the form of methane after the degradation of permafrost. In addition to microbial action, geological methane (metastable methane hydrate, steady-state methane hydrate, and thermogenic methane produced in deep underground or coal seams) stored in the frozen layer of permafrost regions is gradually released. Finally, based on field monitoring results, the thermal gas–solid coupling model of geological methane in the permafrost region is presented, which provides data and technical support for the study of the carbon cycle in the permafrost region in Northeast China.

     

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