Characteristics of Spatial and Temporal Distributions of Methane over the Tibetan Plateau and Mechanism Analysis for High Methane Concentration in Summer
-
摘要: 利用搭载在美国Aqua卫星上的大气红外探测仪(AIRS)观测资料反演的全球甲烷(CH4)产品和NCEP再分析资料,分析了2003~2014年青藏高原上空CH4的时空变化特征,探讨了夏季CH4高值变化与季风的关系。研究结果表明:就青藏高原整体而言,CH4浓度随高度增加递减;对流层中高层CH4含量季节变化较为明显,其平均浓度在7~9月处于高值,6月、10月次之,其余月份处于低值。2003~2014年CH4含量呈逐年上升趋势,年增长率约为4.66ppb(10-9)。高原上空CH4空间分布分析显示,高原北部CH4浓度高于南部地区。夏季风期间,随着高原上的强对流输送和上空南亚高压的阻塞,对流层中高层CH4浓度明显增加并不断积累,在8月底至9月初出现最大值。在分析季风指数的基础上发现,夏季季风影响下的强对流输送是高原对流层中高层CH4高值形成的主要原因之一,对流层中高层CH4浓度最大值出现时间较季风指数的峰值滞后约半至一个月,随着夏季风的撤退,CH4浓度高值迅速降低。
-
关键词:
- 甲烷 /
- 大气红外探测仪(AIRS) /
- 青藏高原 /
- 时空分布 /
- 季风指数
Abstract: Observations of global methane inversion (CH4) products measured middle-upper by the Atmospheric Infrared Sounder (AIRS) on the Aqua satellite and the NCEP reanalysis data are used to investigate characteristic changes in CH4 over the Tibetan Plateau from 2003 to 2014. The relationship between the CH4 change and the monsoon is explored. The results indicate that, taking the Tibetan Plateau as whole, the concentration of CH4 decreases with the increase in altitude. The seasonal variation of CH4 in the middle-upper troposphere is significant. Monthly average concentration of CH4 is the highest from July to September, followed by that in June and October, and the value is low in other months. The concentration of CH4 increased year by year during 2003-2014, showing an overall increasing trend with an annual growth rate of about 4.66ppb (10-9). Based on analysis of the spatial distribution of CH4 over the plateau, the concentration of CH4 is higher in the north than in the south of the plateau. During the summer monsoon period, CH4 concentration in the mid-upper troposphere significantly increases and continues to accumulate due to strong convective transport and influences of South Asia high blocking over the plateau. The maximum CH4 concentration appears at the end of August to early September. Analysis of the monsoon index suggests that strong convection under the influence of summer monsoon is one of the major factors contributing to the high value of CH4 over the Tibetan Plateau. The maximum CH4 concentration appears about one month later than the Monsoon Index. With the decline of the monsoon, the high value of CH4 also quickly decreases. -
图 3 2003~2014年青藏高原300 hPa处CH4平均浓度的年际变化(灰色实线为2003~2014趋势,黑色虚线为2003~2010年趋势,黑色点线为2011~2014年趋势)
Figure 3. Interannual variations of averaged CH4 concentration at 300 hPa over the Tibetan Plateau from 2003 to 2014 (the grey spot solid line represents the growth trend of CH4 concentration from 2003 to 2014, the black solid line represents the growth trend of CH4 concentration from 2003 to 2010, the black dotted line represents the growth trend of CH4 concentration from 2011 to 2014)
表 1 不同季节青藏高原及周边同纬度地区300 hPa处CH4平均浓度
Table 1. Averaged CH4 concentrations at 300 hPa over the Tibetan Plateau and the surrounding area of the same latitude in different seasons
300 hPa处CH4平均浓度(×10–9) 青藏高原区域 周边同纬度陆地区域 春季 1784 1789 夏季 1822 1822 秋季 1817 1822 冬季 1787 1797 -
[1] 白虎志, 谢金南, 李栋梁. 2001.近40年青藏高原季风变化的主要特征[J].高原气象, 20(1):22-27. doi: 10.3321/j.issn:1000-0534.2001.01.004Bai Huzhi, Xie Jinnan, Li Dongliang. 2001. The principal feature of Qinghai-Xizang Plateau monsoon variation in 40 years[J]. Plateau Meteorology (in Chinese), 20(1):22-27, doi: 10.3321/j.issn:1000-0534.2001.01.004. [2] 毕云, 陈月娟, 周任君, 等. 2008.青藏高原上空H2O和CH4的分布和变化趋势分析[J].高原气象, 27(2):249-258.Bi Yun, Chen Yuejuan, Zhou Renjun, et al. 2008. Study on H2O and CH4 distributions and variations over Qinghai-Xizang Plateau using HALOE data[J]. Plateau Meteorology (in Chinese), 27(2):249-258. [3] 程洁, 柳钦火, 李小文. 2007.星载高光谱红外传感器反演大气痕量气体综述[J].遥感信息, (2):90-97. doi: 10.3969/j.issn.1000-3177.2007.02.021Cheng Jie, Liu Qinhuo, Li Xiaowen. 2007. Review of trace gases inversion utilizing space-borne hyperspectral infrared remote sensor data[J]. Remote Sensing Information (in Chinese), (2):90-97, doi:10.3969/j.issn.1000-3177. 2007.02.021. [4] 段安民, 吴国雄, 张琼, 等. 2006.青藏高原气候变暖是温室气体排放加剧结果的新证据[J].科学通报, 51(8):989-992. doi: 10.1007/s11434-006-1396-6Duan Anmin, Wu Guoxiong, Zhang Qiong, et al. 2006. New proofs of the recent climate warming over the Tibetan Plateau as a result of the increasing greenhouse gases emissions[J]. Chinese Science Bulletin, 51(11):1396-1400, doi: 10.1007/s11434-006-1396-6. [5] 高文华, 赵凤生, 盖长松. 2006.大气红外探测器(AIRS)温、湿度反演产品的有效性检验及在数值模式中的应用研究[J].气象学报, 64(3):271-280. doi: 10.11676/qxxb2006.026Gao Wenhua, Zhao Fengsheng, Gai Changsong. 2006. Validation of AIRS retrieval temperature and moisture products and their application in numerical models[J]. Acta Meteorologica Sinicia (in Chinese), 64(3):271-280, doi: 10.11676/qxxb2006.026. [6] Lawrence M G, Rasch P J, von Kuhlmann R, et al. 2003. Global chemical weather forecasts for field campaign planning:Predictions and observations of large-scale features during MINOS, CONTRACE, and INDOEX[J]. Atmospheric Chemistry and Physics, 3(1):267-289, doi: 10.5194/acp-3-267-2003. [7] 李建平, 曾庆存. 2005.一个新的季风指数及其年际变化和与雨量的关系[J].气候与环境研究, 10(3):351-365. doi: 10.3878/j.issn.1006-9585.2005.03.09Li Jianping, Zeng Qingcun. 2005. A new monsoon index, its interannual variability and relation with monsoon precipitation[J]. Climatic and Environmental Research (in Chinese), 10(3):351-365, doi: 10.3878/j.issn.1006-9585.2005.03.09. [8] Li Q B, Jacob D J, Logan J A, et al. 2001. A tropospheric ozone maximum over the Middle East[J]. Geophys. Res. Lett., 28(17):3235-3238, doi: 10.1029/2001GL013134. [9] Liu Y, Li W L, Zhou X J, et al. 2003. The possible influences of the increasing anthropogenic emissions in India on tropospheric ozone and OH[J]. Advances in Atmospheric Science, 20(6):968-977, doi: 10.1007/BF02915520. [10] Milich L. 1999. The role of methane in global warming:where might mitigation strategies be focused?[J]. Global Environmental Change, 9(3):179-201, doi: 10.1016/S0959-3780(98)00037-5. [11] 汤懋苍, 梁娟, 邵明镜, 等. 1984.高原季风年际变化的初步分析[J].高原气象, 3(3):76-82. http://www.cnki.com.cn/Article/CJFDTOTAL-GYQX198403008.htmTang Maocang, Liang Juan, Shao Mingjing, et al. 1984. A preliminary analysis of the interannual variation of the monsoon over the plateau[J]. Plateau Meteorology (in Chinese), 3(3):76-82. http://www.cnki.com.cn/Article/CJFDTOTAL-GYQX198403008.htm [12] 王红梅, 李佳田, 张莹, 等. 2015.利用AIRS产品分析中国地区近地面甲烷浓度时空特性[J].遥感学报, 19(5):827-835. doi: 10.11834/jrs.20154195Wang Hongmei, Li Jiatian, Zhang Ying, et al. 2015. Spatial and temporal distribution of near-surface methane concentration over China based on AIRS observations[J]. Journal of Remote Sensing (in Chinese), 19(5):827-835, doi: 10.11834/jrs.20154195. [13] Xiong X, Houweling S, Wei J, et al. 2009. Methane plume over south Asia during the monsoon season:Satellite observation and model simulation[J]. Atmospheric Chemistry and Physics, 9(3):783-794, doi: 10.5194/acp-9-783-2009. [14] Xiong X Z, Barnet C, Maddy E, et al. 2008. Characterization and validation of methane products from the atmospheric infrared sounder (AIRS)[J]. J. Geophys. Res., 113(G3):G00A01, doi: 10.1029/2007JG000500. [15] 熊效振, 张莹, 陈良富, 等. 2011.季风影响下的青藏高原上空甲烷、水汽及云的变化[J].成都信息工程学院学报, 26(5):480-485. doi: 10.3969/j.issn.1671-1742.2011.05.003Xiong Xiaozhen, Zhang Ying, Chen Liangfu, et al. 2011. Variation of methane, water vapor and clouds over Tibetan Plateau under the impact of Asian summer monsoon[J]. Journal of Chengdu University of Information Technology (in Chinese), 26(5):480-485, doi:10.3969/j.issn.1671-1742. 2011.05.003. [16] Ye D Z, Wu G X. 1998. The role of the heat source of the Tibetan Plateau in the general circulation[J]. Meteor. Atmos. Phys., 67(1-4):181-198, doi: 10.1007/BF01277509. [17] 张剑波. 1996.大气中甲烷的化学行为[J].环境科学研究, 9(4):10-15. http://www.cnki.com.cn/Article/CJFDTOTAL-HJKX199604004.htmZhan Jianbo. 1996. Chemical behavior of methane in atmosphere[J]. Research of Environmental Sciences (in Chinese), 9(4):10-15. http://www.cnki.com.cn/Article/CJFDTOTAL-HJKX199604004.htm [18] Zhang X Y, Bai W G, Zhang P, et al. 2011. Spatiotemporal variations in mid-upper tropospheric methane over China from satellite observations[J]. Chinese Science Bulletin, 56(31):3321-3327, doi: 10.1007/s11434-011-4666-x. [19] 赵玉成, 刘鹏, 王剑琼, 等. 2014. 1991~2011年瓦里关全球大气本底监测事实[J].青海环境, 24(1):32-35. doi: 10.3969/j.issn.1007-2454.2014.01.006Zhao Yucheng, Liu Peng, Wang Jianqiong, et al. 2014. Waliguan global atmospheric background monitoring from 1991 to 2011[J]. Journal of Qinghai Environment (in Chinese), 24(1):32-35, doi: 10.3969/j.issn.1007-2454.2014.01.006. -