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香河地基观测臭氧柱总量数据分析及臭氧变化趋势研究

窦鑫 张金强 朱彬 郑向东 夏祥鳌 陈洪滨

窦鑫, 张金强, 朱彬, 郑向东, 夏祥鳌, 陈洪滨. 香河地基观测臭氧柱总量数据分析及臭氧变化趋势研究[J]. 气候与环境研究, 2019, 24(2): 143-151. doi: 10.3878/j.issn.1006-9585.2018.17102
引用本文: 窦鑫, 张金强, 朱彬, 郑向东, 夏祥鳌, 陈洪滨. 香河地基观测臭氧柱总量数据分析及臭氧变化趋势研究[J]. 气候与环境研究, 2019, 24(2): 143-151. doi: 10.3878/j.issn.1006-9585.2018.17102
Xin DOU, Jinqiang ZHANG, Bin ZHU, Xiangdong ZHENG, Xiangao XIA, Hongbin CHEN. Analysis of Total Ozone Column from Ground-Based Observation and Its Trend at Xianghe Station[J]. Climatic and Environmental Research, 2019, 24(2): 143-151. doi: 10.3878/j.issn.1006-9585.2018.17102
Citation: Xin DOU, Jinqiang ZHANG, Bin ZHU, Xiangdong ZHENG, Xiangao XIA, Hongbin CHEN. Analysis of Total Ozone Column from Ground-Based Observation and Its Trend at Xianghe Station[J]. Climatic and Environmental Research, 2019, 24(2): 143-151. doi: 10.3878/j.issn.1006-9585.2018.17102

香河地基观测臭氧柱总量数据分析及臭氧变化趋势研究

doi: 10.3878/j.issn.1006-9585.2018.17102
基金项目: 

国家重点研发计划项目 2017YFA0603504

中国科学院战略性先导科技专项 XDA17010101

国家自然科学基金项目 61327810

详细信息
    作者简介:

    窦鑫, 男, 1993年出生, 硕士, 主要从事大气环境探测研究。E-mail:1063739203@qq.com

    通讯作者:

    张金强, E-mail:zjq@mail.iap.ac.cn

  • 中图分类号: P412.293

Analysis of Total Ozone Column from Ground-Based Observation and Its Trend at Xianghe Station

Funds: 

National Key Research and Development Program of China 2017YFA0603504

Strategic Priority Research Program of the Chinese Academy of Sciences XDA17010101

National Natural Science Foundation of China 61327810

  • 摘要: 大气臭氧变化在全球气候和环境中具有重要作用,是当今大气科学领域的重要研究对象之一。对比分析了中国科学院大气物理研究所河北香河大气综合观测试验站2014~2016年Dobson和Brewer两种臭氧总量观测仪器探测结果的一致性,并使用1979~2016年Dobson观测数据分析了香河地区臭氧总量的长期变化趋势。结果表明:进行有效温度修正后,两种臭氧总量仪器观测结果一致性较好,平均偏差仅为-0.14 DU(多布森单位),平均绝对偏差为8.00 DU,标准差为36.09 DU,相关系数达0.964。整体来说,两类仪器观测臭氧总量吻合较好。SO2浓度对Dobson仪器数据精度有一定影响,两组仪器数据在SO2浓度为0~0.2 DU、0.2~0.4 DU和>0.4 DU大气条件情况下的平均偏差分别为4.8 DU、7.0 DU和8.0 DU,平均偏差随SO2浓度升高而增大。过去38年香河地区的臭氧总量季节差异性强,春、冬两季臭氧总量高,夏、秋两季臭氧总量相对低,季节变化趋势差异明显。从长期变化上看,臭氧总量变化波动有不同的周期,在4个大的时间段变化趋势不同,2000~2010年臭氧层有显著恢复,但最近几年又有变薄的趋势。
  • 图  1  2014~2016年香河站Dobosn和Brewer匹配观测臭氧总量数据散点图:(a)有效温度订正前;(b)有效温度订正后

    Figure  1.  Scatter plots of total ozone amounts between Dobson and Brewer measurement observations at Xianghe station during 2014–2016: (a) Before effective temperature correction; (b) after effective temperature correction

    图  2  2014~2016年香河站Dobson和Brewer观测臭氧总量时间序列分布及偏差:(a)2014年;(b)2015年;(c)2016年

    Figure  2.  Time series of the total ozone amounts from Dobson and Brewer measurements and their deviations at Xianghe station during 2014–2016: (a) 2014; (b) 2015; (c) 2016

    图  3  2014~2016年SO2浓度为(a)0~0.2 DU、(b)0.2~0.4 DU和(c)>0.4 DU大气条件下香河站Dobson和Brewer匹配观测臭氧总量数据对比

    Figure  3.  Scatter plots of total ozone amounts between Dobson and Brewer observations at Xianghe station during 2014–2016, with the SO2 concentrations of (a) 0–0.2 DU, (b) 0.2–0.4 DU, and (c) > 0.4DU, separately

    图  4  1979~2016年香河站Dobson观测(a)月平均臭氧总量及(b)其变化趋势

    Figure  4.  (a) Dobson measurement monthly averaged total ozone amount, and (b) its variation trend at Xianghe station during 1979–2016

    图  5  1979~2016年香河站Dobson观测臭氧总量数据年平均时间序列

    Figure  5.  Time series of annual mean total ozone amounts from Dobson observation data at Xianghe station during 1979–2016

    表  1  3种仪器观测次数和累计天数

    Table  1.   Observational numbers and days of the instruments

    仪器 每天测量次数 累计天数/d 观测时间段
    Dobson ≤5 550 2014年1月至2016年12月
    Brewer 多次 550
    MAX-DOAS 多次 300
    下载: 导出CSV

    表  2  2014~2016年香河站Dobosn和Brewer匹配观测臭氧总量数据结果

    Table  2.   Results of matched total ozone amounts from Dobson and Brewer measurements at Xianghe station during 2014–2016

    平均偏差/DU 平均绝对偏差/DU 标准差/DU 相关系数 样本数
    有效温度订正前 −0.39 8.73 35.73 0.959 1404
    有效温度订正后 −0.14 8.00 36.09 0.964 1404
    下载: 导出CSV

    表  3  2014~2016年香河站Dobosn和Brewer日平均匹配臭氧总量数据结果

    Table  3.   Daily average results of matched total ozone amounts from Dobson and Brewer measurements at Xianghe station during 2014–2016

    平均偏差/DU 平均绝对偏差/DU 标准差/DU 相关系数 样本数
    0.91 7.41 34.68 0.969 550
    下载: 导出CSV

    表  4  2014~2016年3类SO2大气条件下Dobson和Brewer匹配观测臭氧总量数据对比

    Table  4.   Comparison of matched total ozone amount observations between Dobson and Brewer under three types of SO2 atmospheric conditions

    平均偏差/DU 平均绝对偏差/DU 标准差/DU 相关系数 匹配样本数
    SO2浓度0~0.2 DU 4.8 6.1 30.4 0.98 102
    SO2浓度0.2~0.4 DU 7.0 7.7 37.6 0.98 74
    SO2浓度>0.4 DU 8.0 8.5 32.8 0.98 124
    下载: 导出CSV
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  • 收稿日期:  2017-07-17
  • 网络出版日期:  2018-03-21
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