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德庆卓嘎, 高佳佳, 白志宣, 等. 2024. 拉萨市近地面大气成分时空变化及相关因子研究[J]. 气候与环境研究, 29(2): 125−135. doi: 10.3878/j.issn.1006-9585.2023.22126
引用本文: 德庆卓嘎, 高佳佳, 白志宣, 等. 2024. 拉萨市近地面大气成分时空变化及相关因子研究[J]. 气候与环境研究, 29(2): 125−135. doi: 10.3878/j.issn.1006-9585.2023.22126
DEQING Zhuoga, GAO Jiajia, BAI Zhixuan, et al. 2024. Study on Spatiotemporal Changes and Related Factors of Near-Surface Atmospheric Composition in Lhasa City [J]. Climatic and Environmental Research (in Chinese), 29 (2): 125−135. doi: 10.3878/j.issn.1006-9585.2023.22126
Citation: DEQING Zhuoga, GAO Jiajia, BAI Zhixuan, et al. 2024. Study on Spatiotemporal Changes and Related Factors of Near-Surface Atmospheric Composition in Lhasa City [J]. Climatic and Environmental Research (in Chinese), 29 (2): 125−135. doi: 10.3878/j.issn.1006-9585.2023.22126

拉萨市近地面大气成分时空变化及相关因子研究

Study on Spatiotemporal Changes and Related Factors of Near-Surface Atmospheric Composition in Lhasa City

  • 摘要: 拉萨市位于青藏高原腹地,近年来臭氧(O3)污染问题凸显。本文基于2013~2018年拉萨市区6个监测站点的O3、NO、NO2、NOx、CO、SO2、PM2.5、PM10监测数据,采用相关统计方法研究了拉萨市各污染物,尤其是O3的时空分布特征及与前体物之间关系,并探讨了气象条件对其的影响。结果表明:(1)近年来拉萨市区O3浓度呈上升趋势,O3替代PM10,成为拉萨城区首要污染物。O3浓度的年超标天数达55 d,占比为49.4%。(2)O3浓度在2016年之后上升显著,上升率为16.34 μg m−3 a−1,2018年O3浓度最大(91.48 μg/m3);年较差计算得出,每年生成的O3浓度从2015年开始逐渐升高。(3)O3浓度呈现春高冬低,城区高于郊区的变化特征,且与NO、NO2和NOx的浓度变化存在显著的负相关关系(-0.6),可能O3生成被NOx抑制。(4)O3浓度与气温相关性较好,随着降水量和湿度的增加,抑制O3浓度增加。O3浓度受季节和风向风速影响较大,这可能与长距离传输特征及人类活动(固定源)对高原生态环境影响有关。

     

    Abstract: Lhasa City is located in the hinterland of the Qinghai–Tibet Plateau. The problem of ozone (O3) pollution has become significant in recent years. Based on the monitoring data of O3, NO, NO2, NOx, CO, SO2, PM2.5, and PM10 from six monitoring stations in the Lhasa urban area from 2013 to 2018, this paper uses statistical methods to study various pollutants in Lhasa. This especially includes the temporal and spatial distribution characteristics of O3, the relationship between ozone and its precursors, and the influence of meteorological conditions on ozone.The results show that (1) O3 concentration in the Lhasa urban area has been increasing in recent years. Further, O3 replaces PM10 as the primary pollutant in the Lhasa urban area. Additionally, the annual days of excess O3 have reached 55 d, accounting for 49.4% of the total days. (2) The O3 concentration has increased significantly after 2016, with an increasing rate of 16.34 μg m-3 a-1 from 2016 to 2018, and the O3 concentration is the highest in 2018 (91.48 μg/m3). The annual difference in the ozone concentration shows that the annual O3 concentration has gradually increased since 2015. (3) The O3 concentration increases in spring and decreases in winter; furthermore, the urban area has a higher O3 concentration than the suburban area, and it is negatively correlated with the concentration of NO, NO2, and NOx (−0.6). Therefore, it is possible that ozone generation is inhibited by NOx. (4) O3 correlates well with air temperature; therefore, with an increase in precipitation and humidity, the O3 concentration is inhibited. Furthermore, the O3 concentration is greatly affected by the season and wind direction and speed. These factors can be related to the characteristics of long-distance transport and the impact of human activities (stationary sources) on the plateauing ecological environment.

     

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