Abstract:
To systematically reveal the characteristics of atmospheric pollutant emissions from agricultural sources in the Yangtze River Delta region, this study developed a comprehensive 4 km high-resolution agricultural emission inventory for the period 2012-2018, covering agricultural machinery, farmland soil dust, farmland soil NO, open straw burning, and agricultural ammonia. The results show that the annual average emissions of agricultural PM
10, PM
2.5, THC, NO
x, CO, SO
2, and NH
3 were 61.5 Gg yr-1, 54.1 Gg yr-1, 74.2 Gg yr-1, 258.2 Gg yr-1, 644.0 Gg yr-1, 4.8 Gg yr-1, and 1302.2 Gg yr-1, respectively. Spatially, emissions were highly concentrated in the agricultural areas of northern Jiangsu and northern Anhui. Temporally, emissions showed a pattern of higher levels in summer and autumn and lower levels in winter and spring. From 2012 to 2018, emissions of all pollutants showed a declining trend: PM
10, PM
2.5, CO, and THC decreased sharply by 73.1%–84.5%, mainly attributable to the effective implementation of straw burning bans; SO
2 and NO? declined rapidly but slightly more slowly than the first group (by 60.8% and 48.7%, respectively); NH
3 decreased slowly and steadily (by 16.1%). Meanwhile, the structure of agricultural emissions underwent significant transformation, with agricultural machinery replacing straw burning as the primary contributor to PM
10, PM
2.5, NO
x, CO, THC, and SO
2, and its contribution to NO? consistently remained above 80%. The contributions from farmland soil dust and soil NO emissions increased significantly. The study results provide a scientific basis and data support for atmospheric pollution control.